If you have an S2 or TC/S, then by all means, use dynamat (or equivalent). Make sure anything you use inside the engine compartment is rated for that use due to the risk of engine fires.
On an S1 the massive curved sections leading to the hollow sills act like two giant flugelhorns. The chassis is riveted solid to the body. Noise is just part of the package.
I lined both sides of my S1's firewall with a dynamat equivalent and fit a sheet of aluminium as well.The rest of the interior was also lined with sound deadening. It's unbelievably, laugh-out-loud, LOUD. It's actually kind of cool for an hour. After that, not so much. I use Bose aviation, noise-cancelling headsets and a comm system for any trips.